Multimodal systems are a workaround to enhance the robustness and effectiveness of biometric systems. A proper multimodal dataset is of the utmost importance to build such systems. The literature presents some multimodal datasets, although, to the best of our knowledge, there are no previous studies combining face, iris/eye, and vital signals such as the Electrocardiogram (ECG). Moreover, there is no methodology to guide the construction and evaluation of a chimeric dataset. Taking that fact into account, we propose to create a chimeric dataset from three modalities in this work: ECG, eye, and face. Based on the criteria, we also propose a generic and systematic protocol imposing constraints for the creation of homogeneous chimeric individuals, which allow us to perform a fair and reproducible benchmark. Moreover, we have proposed a multimodal approach for these modalities based on state-of-the-art deep representations built by convolutional neural networks. We conduct the experiments in the open-world verification mode and on two different scenarios (intra-session and inter-session), using three modalities from two datasets: CYBHi (ECG) and FRGC (eye and face). Our multimodal approach achieves impressive decidability of 7.20 ± 0.18, yielding an almost perfect verification system (i.e., Equal Error Rate (EER) of 0.20% ± 0.06) on the intra-session scenario with unknown data. On the inter-session scenario, we achieve a decidability of 7.78 ± 0.78 and an EER of 0.06% ± 0.06. In summary, these figures represent a gain of over 28% in decidability and a reduction over 11% of the EER on the intra-session scenario for unknown data compared to the best-known unimodal approach. Besides, we achieve an improvement greater than 22% in decidability and an EER reduction over 6% in the inter-session scenario.