number size distributions and seasonality of submicron particles in europe 2008–2009

number size distributions and seasonality of submicron particles in europe 2008–2009

;A. Asmi;A. Wiedensohler;P. Laj;A.-M. Fjaeraa;K. Sellegri;W. Birmili;E. Weingartner;U. Baltensperger;V. Zdimal;N. Zikova;J.-P. Putaud;A. Marinoni;P. Tunved;H.-C. Hansson;M. Fiebig;N. Kivekäs;H. Lihavainen;E. Asmi;V. Ulevicius;P. P. Aalto;E. Swietlicki;A. Kristensson;N. Mihalopoulos;N. Kalivitis;I. Kalapov;G. Kiss;G. de Leeuw;B. Henzing;R. M. Harrison;D. Beddows;C. O'Dowd;S. G. Jennings;H. Flentje;K. Weinhold;F. Meinhardt;L. Ries;M. Kulmala
Journal of agricultural and food chemistry 2011 Vol. 11 pp. 5505-5538
111
asmi2011atmosphericnumber

Abstract

Two years of harmonized aerosol number size distribution data from 24 European field monitoring sites have been analysed. The results give a comprehensive overview of the European near surface aerosol particle number concentrations and number size distributions between 30 and 500 nm of dry particle diameter. Spatial and temporal distribution of aerosols in the particle sizes most important for climate applications are presented. We also analyse the annual, weekly and diurnal cycles of the aerosol number concentrations, provide log-normal fitting parameters for median number size distributions, and give guidance notes for data users. Emphasis is placed on the usability of results within the aerosol modelling community. <br></br> We also show that the aerosol number concentrations of Aitken and accumulation mode particles (with 100 nm dry diameter as a cut-off between modes) are related, although there is significant variation in the ratios of the modal number concentrations. Different aerosol and station types are distinguished from this data and this methodology has potential for further categorization of stations aerosol number size distribution types. <br></br> The European submicron aerosol was divided into characteristic types: Central European aerosol, characterized by single mode median size distributions, unimodal number concentration histograms and low variability in CCN-sized aerosol number concentrations; Nordic aerosol with low number concentrations, although showing pronounced seasonal variation of especially Aitken mode particles; Mountain sites (altitude over 1000 m a.s.l.) with a strong seasonal cycle in aerosol number concentrations, high variability, and very low median number concentrations. Southern and Western European regions had fewer stations, which decreases the regional coverage of these results. Aerosol number concentrations over the Britain and Ireland had very high variance and there are indications of mixed air masses from several source regions; the Mediterranean aerosol exhibit high seasonality, and a strong accumulation mode in the summer. The greatest concentrations were observed at the Ispra station in Northern Italy with high accumulation mode number concentrations in the winter. The aerosol number concentrations at the Arctic station Zeppelin in Ny-AA lesund in Svalbard have also a strong seasonal cycle, with greater concentrations of accumulation mode particles in winter, and dominating summer Aitken mode indicating more recently formed particles. Observed particles did not show any statistically significant regional work-week or weekday related variation in number concentrations studied. <br></br> Analysis products are made for open-access to the research community, available in a freely accessible internet site. The results give to the modelling community a reliable, easy-to-use and freely available comparison dataset of aerosol size distributions.

Citation

ID: 243216
Ref Key: asmi2011atmosphericnumber
Use this key to autocite in SciMatic or Thesis Manager

References

Blockchain Verification

Account:
NFT Contract Address:
0x95644003c57E6F55A65596E3D9Eac6813e3566dA
Article ID:
243216
Unique Identifier:
10.5194/acp-11-5505-2011
Network:
Scimatic Chain (ID: 481)
Loading...
Blockchain Readiness Checklist
Authors
Abstract
Journal Name
Year
Title
5/5
Creates 1,000,000 NFT tokens for this article
Token Features:
  • ERC-1155 Standard NFT
  • 1 Million Supply per Article
  • Transferable via MetaMask
  • Permanent Blockchain Record
Blockchain QR Code
Scan with Saymatik Web3.0 Wallet

Saymatik Web3.0 Wallet