In this paper, we studied the frequency of occurrence and shortwave direct
radiative effects (DREs) of above-cloud aerosols (ACAs) over global oceans
using 8 years (2007–2014) of collocated CALIOP and MODIS
observations. Similar to previous work, we found high ACA occurrence in four
regions: southeastern (SE) Atlantic region, where ACAs are mostly
light-absorbing aerosols, i.e., smoke and polluted dust according to CALIOP
classification, originating from biomass burning over the African Savanna;
tropical northeastern (TNE) Atlantic and the Arabian Sea, where ACAs are predominantly
windblown dust from the Sahara and Arabian deserts, respectively; and
the northwestern (NW) Pacific, where ACAs are mostly transported smoke and polluted dusts
from Asian. From radiative transfer simulations based on CALIOP–MODIS
observations and a set of the preselected aerosol optical models, we found
the DREs of ACAs at the top of atmosphere (TOA) to be positive (i.e.,
warming) in the SE Atlantic and NW Pacific regions, but negative (i.e.,
cooling) in the TNE Atlantic Ocean and the Arabian Sea. The cancellation of positive and
negative regional DREs results in a global ocean annual mean diurnally
averaged cloudy-sky DRE of 0.015 W m
−2 (range of −0.03 to 0.06 W m
−2) at TOA. The DREs at surface and within the atmosphere are
−0.15 W m
−2 (range of −0.09 to −0.21 W m
−2), and 0.17 W m
−2 (range
of 0.11 to 0.24 W m
−2), respectively. The regional and seasonal mean
DREs are much stronger. For example, in the SE Atlantic region, the JJA
(July–August) seasonal mean cloudy-sky DRE is about 0.7 W m
−2
(range of 0.2 to 1.2 W m
−2) at TOA. All our DRE computations are
publicly
available
1.
The uncertainty in our DRE computations is mainly caused by the uncertainties
in the aerosol optical properties, in particular aerosol absorption, the
uncertainties in the CALIOP operational aerosol optical thickness retrieval,
and the ignorance of cloud and potential aerosol diurnal cycle. In situ and
remotely sensed measurements of ACA from future field campaigns and
satellite missions and improved lidar retrieval algorithm, in particular
vertical feature masking, would help reduce the uncertainty.
1 https://drive.google.com/folderview?id=0B6gKx4dgNY0GMVYzcEd0bkZmRmc&usp=sharing