real-time observation of ultrafast rabi oscillations between excitons and plasmons in metal/molecular aggregate hybrid nanostructures
;Cerullo G.;Manzoni C.;Maiuri M.;Lammers M.;Pomraenke R.;Vasa P.;Wang W.;Lienau C.
utilitas mathematica2013Vol. 41pp. 09018-
178
g.2013epjreal-time
Abstract
We demonstrate ultrafast coherent manipulation of the normal mode splitting in metal/molecular-aggregate nanostructures by real-time observation of Rabi oscillations between excitons and surface-plasmon-polaritons. Oscillations in exciton density on a 10-fs timescale control the Rabi splitting.