Discovery and Biosynthesis of Neoenterocins Indicate a Skeleton Rearrangement of Enterocin.
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Discovery and Biosynthesis of Neoenterocins Indicate a Skeleton Rearrangement of Enterocin.

Zheng, Liujuan;Jiang, Xiaodong;Zhang, Qingbo;Zhu, Yiguang;Zhang, Haibo;Zhang, Wenjun;Saurav, Kumar;Liu, Jinsong;Zhang, Changsheng;
Organic letters 2019 Vol. 21 pp. 9066-9070
227
zheng2019discoveryorganic

Abstract

Two polyketides neoenterocins A () and B (), featuring a neighboring dicarbonyl motif and a furan-containing 5/6 ring system, were isolated from the enterocin producer sp. SCSIO 11863. Heterologous expression, gene disruptions, and isotope feeding experiments indicated that and were derived from the enterocin biosynthetic gene cluster. However, was demonstrated as an artifact from enterocin via a unique skeleton rearrangement.

Keywords

actinobacteria lc-hrms natural product biosynthetic gene clusters (bgcs) cyclic dipeptides (2,5-diketopiperazines, dkps) global natural product social networking (gnps) quorum sensing inhibition (qsi)

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DOI:
10.1021/acs.orglett.9b03460

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