Interplay of arene radical cations with anions and fluorinated alcohols in hole catalysis
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Interplay of arene radical cations with anions and fluorinated alcohols in hole catalysis

Shida, Naoki;Imada, Yasushi;Nagahara, Shingo;Okada, Yohei;Chiba, Kazuhiro;
Communications chemistry 2019 Vol. 2 pp. 1-8
351
shida2019interplaycommunications

Abstract

Fluorinated solvents such as hexafluoroisopropanol (HFIP) are often useful in reactions involving radical cations. Here the role of HFIP in photoredox and electrochemical Diels-Alder reactions is explored experimentally and theoretically, and attributed to solvation of anions to reduce their nucleophilicity.

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