High iso Aldehyde Selectivity in the Hydroformylation of Short-Chain Alkenes.
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High iso Aldehyde Selectivity in the Hydroformylation of Short-Chain Alkenes.

Iu, Leo;Fuentes, José A;Janka, Mesfin E;Fontenot, Kevin J;Clarke, Matthew L;
Angewandte Chemie (International ed. in English) 2019 Vol. 58 pp. 2120-2124
162
iu2019highangewandte

Abstract

The hydroformylation of propene to give predominantly iso-butanal has been achieved; class-leading selectivity is possible even at higher temperatures that deliver fast conversion. Racemic rhodium complexes of bidentate phospholane phosphites derived from tropos-biphenols and unusual solvent systems are the key to the selectivity observed.

Keywords

rhodium enantioselective catalysis fluorinated solvents hydroformylation phosphorus ligands

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DOI:
10.1002/anie.201811888

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ID: 263115
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