Conical-intersection dynamics and ground-state chemistry probed by extreme-ultraviolet time-resolved photoelectron spectroscopy

Conical-intersection dynamics and ground-state chemistry probed by extreme-ultraviolet time-resolved photoelectron spectroscopy

Conta, A. von;Tehlar, A.;Schletter, A.;Arasaki, Y.;Takatsuka, K.;Wörner, H. J.;
Nature communications 2018 Vol. 9 pp. 1-10
226
conta2018conicalintersectionnature

Abstract

Recent progress in extreme-ultraviolet table-top light sources is enabling advances in ultrafast molecular dynamics. Here the authors demonstrate time-resolved photoelectron spectroscopy with such a source, observing how a molecular wave packet crosses a conical intersection, performs large-amplitude motion and eventually dissociates.

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