Conical-intersection dynamics and ground-state chemistry probed by extreme-ultraviolet time-resolved photoelectron spectroscopy
Conta, A. von;Tehlar, A.;Schletter, A.;Arasaki, Y.;Takatsuka, K.;Wörner, H. J.;
Nature communications2018Vol. 9pp. 1-10
226
conta2018conicalintersectionnature
Abstract
Recent progress in extreme-ultraviolet table-top light sources is enabling advances in ultrafast molecular dynamics. Here the authors demonstrate time-resolved photoelectron spectroscopy with such a source, observing how a molecular wave packet crosses a conical intersection, performs large-amplitude motion and eventually dissociates.